Though I don’t think you need much more than a day or two in Zadar (I was actually planning on spending a few days here, and then cut that down to one when I realized how small the city centre was), it’s definitely worth checking out. Maybe as a day trip from nearby Split?
If you’re anywhere in the area, you pretty much have to check out Matera. It’s been continuously occupied since the Palaeolithic era (!), making it the oldest city in Italy and in Europe.